就我个人而言，我喜欢 PyQt4，因为我喜欢 QT4，并且 py2exe 与它配合得很好，wxPython 是另一个好东西，但它在 Windows 下运行得不太好，请参见我的问题：wx.App (wxPython) 调用时崩溃
您可以检查使用各个框架开发的一些应用程序，以及看看有没有你喜欢的。
Pick the one you like, there's no "the best" here.
Personally I like PyQt4, because I like QT4, and py2exe works perfectly fine with it, wxPython is another good thing, but it does not work very well under Windows, see my question here: wx.App (wxPython) crash when calling
You can check some application developed using each frameworks, and see if you like any.
For PyGTK - Glade should be your best bet. Similarly, Rapyd-Tk seems to be good for TK. Though for Tk, I would advise you to try with the articles which help you build from the code and then go with the builders. This answer in SO provides the wealth of options available for building GUI using WxPython.
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选择你喜欢的，这里没有“最好的”。
就我个人而言，我喜欢 PyQt4，因为我喜欢 QT4，并且 py2exe 与它配合得很好，wxPython 是另一个好东西，但它在 Windows 下运行得不太好，请参见我的问题：wx.App (wxPython) 调用时崩溃
您可以检查使用各个框架开发的一些应用程序，以及看看有没有你喜欢的。
Pick the one you like, there's no "the best" here.
Personally I like PyQt4, because I like QT4, and py2exe works perfectly fine with it, wxPython is another good thing, but it does not work very well under Windows, see my question here: wx.App (wxPython) crash when calling
You can check some application developed using each frameworks, and see if you like any.
对于 PyGTK - Glade 应该是你最好的选择。同样，Rapyd-Tk 似乎对 TK 有好处。不过对于 Tk，我建议您尝试使用可帮助您从代码构建的文章，然后与构建器一起使用。 SO 中的这个答案提供了丰富的可用于构建的选项使用 WxPython 的 GUI。
For PyGTK - Glade should be your best bet. Similarly, Rapyd-Tk seems to be good for TK. Though for Tk, I would advise you to try with the articles which help you build from the code and then go with the builders. This answer in SO provides the wealth of options available for building GUI using WxPython.